Carroll County is a county located in the U.S. state of Arkansas. As of the 2020 census, the population was 28,260. The county has two county seats, Berryville and Eureka Springs. Carroll County is Arkansas's 26th county, formed on November 1, 1833, and named after Charles Carroll, the last surviving signer of the United States Declaration of Independ…Carroll County is a county located in the U.S. state of Arkansas. As of the 2020 census, the population was 28,260. The county has two county seats, Berryville and Eureka Springs. Carroll County is Arkansas's 26th county, formed on November 1, 1833, and named after Charles Carroll, the last surviving signer of the United States Declaration of Independence.
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